Dynamics of Interfacial Electron Transfer from Betanin to Nanocrystalline TiO2: The Pursuit of Two-Electron Injection

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Dynamics of Interfacial Electron Transfer from Betanin to Nanocrystalline TiO2: The Pursuit of Two-Electron Injection

We report spectroelectrochemical and transient absorption spectroscopic studies of electron injection from the plant pigment betanin (Bt) to nanocrystalline TiO2. Spectroelectrochemical experiments and density functional theory (DFT) calculations are used to interpret transient absorption data in terms of excited state absorption of Bt and ground state absorption of oxidation intermediates and ...

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ژورنال

عنوان ژورنال: The Journal of Physical Chemistry C

سال: 2015

ISSN: 1932-7447,1932-7455

DOI: 10.1021/acs.jpcc.5b05896